D-127

Product Specific HPLC Method Optimization

Section D — Laboratory Operations and Specifications Revision 1 5 pages

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1.0 Purpose 
 
 The purpose of this procedure is to define the process for optimization of existing HPLC methods
 for specific products. 
 
 2.0 Scope 
 
 This procedure applies to the optimization of existing HPLC methods for specific products that
 are not amenable to analysis using the method as written.. 
 
 3.0 Responsibility 
 
 Sal It is the responsibility of QC Chemists and/or Analytical Development to understand and
 
 work within the guidelines of this procedure. 
 
 3.2 Itis the responsibility of QC Laboratory Management and/or Analytical Development to
 ensure compliance with this procedure and to keep this procedure aligned with current
 
 practices. 
 
 4.0 Definitions 
 
 4.1 QC — Quality Control 
 
 4.2 HPLC — High Performance Liquid Chromatography 
 
 4.3 UV — Ultraviolet Detection 
 
 5.0 References 
 
 5.1 D-126, SOP, Non-Conforming Results in the QC Laboratory 
 
 5.2 C-201, SOP, Deviation and Investigation Procedure 
 
 
 

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 6.0 Overview 
 
 6.1 Because of the large number of products manufactured at Jon Labs, analyte specific
 
 HPLC methods cannot be validated for every product. In some cases, the sample
 
 preparation instructions in an analyte specific HPLC method may not perform as
 expected for a given product. When such a case is identified, a product specific method
 
 optimization may overcome the method deficiency. Product specific method optimization
 may be triggered by certain events including, but not limited to: 
 
 6.1.1 An out of specification test result which was determined to be “Minor” as defined
 
 in D-126 Non-Conforming Results in the QC Laboratory was obtained for either
 
 finished product release or stability testing. 
 
 6.1.2 Anew product, which has not previously undergone testing, is expected to present
 incompatibility with a HPLC method due to a unique characteristic of the product
 
 such as sample matrix, label claim, serving size, or dosage form.
 
 6.2 After successful completion of a product specific method optimization, the Test Details
 section of the product profile will be updated to reflect the method optimization. At a
 
 minimum, the Test Details should include: 
 
 6.2.1 Instructions for preparing the sample in accordance with the optimal conditions.
 
 6.2.2 Instructions for preparing the working standard at the concentration used during
 
 optimization. 
 
 6.2.3 A list of any deviations to the existing method that are required to obtain reliable
 results for the specific product/analyte (e.g. alternate wavelength, injection
 
 volume, or diluent). Any deviation outlined in the Test Details is henceforth no
 longer considered a deviation and does not require documentation by SOP C-201
 
 Deviation and Investigation Procedure. 
 
 6.2.4 If applicable, the maximum time for which the sample preparation is stable.
 
 6.3. The results generated during product specific method optimization shall not be used for
 
 finished product release. To ensure this, the following guidelines will be adhered to:
 
 
 

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 6.3.1 Sequences generated during product specific method optimization shall not be
 
 stored in the same project folder as those generated for finished product release.
 
 6.3.2 Sequence names and sample names for sequences generated during product
 specific method optimization shall not include a batch number. The product name,
 
 formula number, or test identifier (e.g. LOWCONC, MIDCONC, HIGHCONC)
 
 should be used instead. 
 
 6.4 If it is determined that two formulas are sufficiently similar, a single method optimization
 can be performed for the set or a reduced version of the criteria listed herein may be
 
 appropriate. Scientific justification is required. 
 
 7.0 Procedure 
 
 71 Sample preparation and/or method parameters which may need optimization are listed
 
 below. Only Accuracy and Specificity are required. It is up to the discretion of the analyst
 to decide which other parameters may benefit from optimization. 
 
 tee Accuracy 
 
 7.2.1 Spike a placebo with authentic reference standard at a level corresponding to that
 
 expected in the finished product formulation. 
 
 7.2.2 Alternatively: prepare an unspiked sample and a spiked sample, and determine
 the recovery of spiked analyte. Both the spiked and unspiked samples should be
 
 within the linear range of the method. 
 
 Tied Acceptance Criteria 
 
 7.2.3.1 In general, the spike recovery should be within the range 95% - 105%.
 
 More or less stringent acceptance criteria may be used depending on
 product requirements. For example, if the product contains a very small
 
 amount of the target analyte with a large (40%) overage added, an
 acceptance criteria of 90% - 110% may be more appropriate. Scientific
 
 justification is required. 
 
 7.3 Specificity 
 
 
 

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 Taek Using the optimal conditions determined during optimization, the assay should
 
 meet the following criteria for Specificity. 
 
 7.3.2 Acceptance Criteria 
 
 7.3.2.1 The retention time of the target analyte in the sample chromatogram
 differs from that of the reference standard by no more than 0.3 min. If
 
 the retention time is greater than 15 min, then the difference may be no
 
 more than 3%. 
 
 7.3.2.2 For HPLC/UV: The spectral match of the target analyte in the sample
 chromatogram with that of the reference standard is no less than 900.
 
 7.4 Extraction Conditions 
 
 7.4.1 For samples that require extraction: perform the analytical test method using
 
 different extraction conditions. 
 
 7.4.2 Sample preparation may consist of any combination of shaking, stirring, heating,
 and/or sonication. Extraction conditions that may be varied include sonication
 
 time, shaking time, intensity of shaking, stir time, intensity of stirring, extraction
 
 temperature, and/or protection from light. 
 
 7.4.3 The optimal extraction condition is usually the one which results in the highest
 assay value. However, all data collected should be evaluated as a whole to
 
 determine if this is true. For example, a very vigorous extraction condition may
 result in extraction of a previously unobserved interfering compound resulting in
 
 inflated assay value. This would be evident in an unsatisfactory spectral match to
 
 the reference standard. 
 
 7.5 Sample Concentration 
 
 Tol Perform the analytical test method at different sample concentrations within the
 validated linear range of the method. 
 
 dee The optimal sample concentration is usually the one which results in the assay
 
 value with highest percent of label claim. As discussed above, this may not always
 be true. For example, a high sample concentration may result in poor
 
 
 

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 chromatography with co-elution causing overestimation of the assay value. This
 
 would be evident from the chromatography and from reduced spectral match.
 
 7.6 Solution Stability 
 
 7.6.1 For analytes that have been observed to be or are expected to be unstable in
 solution, perform repeat injection of the sample over the course of at least three
 
 hours. 
 
 7.6.2 The composition of the extraction solvent/diluent may require adjustment if
 
 solution stability in the method specified diluent is not sufficient.
 
 76.3 Acceptance Criteria 
 
 7.6.3.1 The sample preparation is stable as long as the change in measured
 concentration does not change relative to the initial concentration by
 
 more than 5.0%. More or less stringent criteria may be used with
 scientific justification as discussed above for Accuracy.
 
 8.0 Revision History 

| Rev | Date | Description of Changes | CCR # | By |
|-----|----------|------------------------|-------|----|
| 0 | 12/20/22 | New procedure N/A S. Sassman A report is no longer required, using a purposely adulterated sample | - | - |
| 1 | 06/06/23 | is no longer required, only specificity and accuracy optimizations CC- will be required. Update logo and format. | 23-0273 | S. Sassman |