D-802

LC-MS Operation Maintenance and Qualification

Section D — Laboratory Operations and Specifications Revision 1 18 pages

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1.0 Purpose 
 
 This procedure provides guidelines for general use, routine maintenance, and performance
 qualification of the Agilent Ultivo LC-MS system. 
 
 2.0 Scope 
 
 This procedure applies to the Agilent Ultivo LC-MS system used in the QC Laboratory at Ion
 Labs. 
 
 3.0 Responsibility 
 3.1 It is the responsibility of QC Laboratory analysts to follow the guidelines for general use
 
 of the Agilent Ultivo LC-MS system. 
 3.2 QC Laboratory Management and/or AD personnel are responsible for ensuring analysts
 follow the guidelines set forth herein. 
 
 3.3 It is the responsibility of QC Laboratory Management, AD personnel, and/or outside
 contractors to perform maintenance and qualification of the Agilent Ultivo LC-MS.
 
 3.4 It is the responsibility of QC Laboratory Management and/or AD personnel to keep this
 SOP current with the latest Ion Labs Practices. 
 
 4.0 Definitions 
 
 4.1 QC — Quality Control 
 
 4.2 AD-—Analytical Development 
 4.3. LC-—Liquid Chromatography 
 
 4.4 MS -— Mass Spectrometry 
 
 4.5 HPLC — High Performance Liquid Chromatography 
 4.6 ESI -—Electrospray Ionization 
 
 4.7 QQQ- Triple Quadrupole Mass Spectrometer 
 48 | MRM — Multiple Reaction Monitoring 
 
 4.9 ISTD-— Internal Standard 
 
 4.10 PTFE — Polytetrafluoroethylene 
 
 
 

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 4.11 DA-— Data Analysis 
 
 4.12 IQ -Installation Qualification 
 
 4.13 OQ- Operational Qualification 
 4.14 PQ- Performance Qualification 
 
 5.0 References 
 
 Da D-602, SOP, Labeling and Expiration Dating of Laboratory Chemicals
 
 5.2 D-603, SOP, Chemical Waste Disposal 
 5.3 D-807, SOP, HPLC Operation, Maintenance, and Qualification. 
 
 5.4 Agilent Ultivo Triple Quadrupole LC-MS Concepts Guide 
 
 Dia) Agilent Ultivo Triple Quadrupole LC-MS System Quick Start Guide 
 5.6 Agilent MassHunter Workstation Software Quantitative Analysis Familiarization Guide
 
 6.0 Safety Precautions 
 
 6.1 Solvents used as mobile phases are toxic and flammable. The minimum required personal
 protective equipment includes safety glasses, gloves, and enclosed shoes. Ensure that
 solvent reservoirs and waste containers are gas-tight. 
 
 6.2 HPLC systems operate at high pressure. Compressed liquids may cause eye injury if a
 sudden leak occurs. 
 
 6.3 The spray chamber drain tube and exhaust tube must be vented externally to the building
 (e.g. into a fume hood). 
 
 6.4 The vacuum pump exhaust tube must be vented externally to the building (e.g. into a
 fume hood). 
 
 6.5 Electrical faults could cause electrocution, explosion or fire. If an electrical fault is
 suspected, disconnect power from the instrument and have it serviced by a qualified
 individual. 
 
 7.0 Waste Handling and Disposal 
 
 7.1 Waste handling and disposal procedures are outlined in SOP D-603 Chemical Waste
 Disposal. 
 8.0 General Guidelines 
 
 8.1 For guidance on general use and maintenance of HPLC systems, consult SOP D-807
 HPLC Operation, Maintenance, and Qualification Documentation. 
 
 8.2 The following parameters should be recorded in the laboratory notebook:
 
 

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 8.2.1 Instrument lon Number 
 
 8.2.2 Instrument Cal Due Date 
 8.2.3 Column identifier 
 
 8.3. Use only LC-MS grade solvents and reagents. The use of solvents and reagents of lower
 purity will result in high background and decreased sensitivity. 
 
 8.4 Use only volatile mobile phase additives such as formic acid, acetic acid, ammonium
 formate, ammonium carbonate, triethylamine, and tridecafluoroheptanoic acid.
 
 8.5 The bench that the Ultivo system sits on must be sturdy enough to hold the weight of the
 mass spectrometer and HPLC system (up to 275 Ibs). 
 
 8.6 Do not attempt to move the mass spectrometer or HPLC system. 
 
 8.7. Ensure sufficient space for ventilation (min 6 inches on all sides).
 8.8 The drain bottle should sit below the mass spectrometer and be connected to the ion
 
 source by a hose. 
 8.9 Make sure the leak drain connector on the lower right side of the mass spectrometer
 connects to a drain bottle. 
 
 8.10 Nitrogen (minimum 95.0% pure) is the only acceptable drying and nebulizing gas. Use
 of air, oxygen, or other gases, when combined with volatile solvents and high
 voltages in the spray chamber, can result in an explosion. Use of air, oxygen, or other
 
 gases also causes deterioration of parts in the Ultivo LC/TQ and 
 negatively impacts instrument operation and sensitivity. Less than 0.1 ppm of
 hydrocarbons with the remaining gas must be oxygen and trace argon. At least 3 L/min
 is required at all times to prevent air from entering the mass spectrometer.
 
 8.11 The stack on top of the mass spectrometer should not be taller than 30 inches. Make sure
 that solvent bottles at the top of the stack can be reached safely.
 
 8.12 The spray chamber exhaust must not have positive pressure. Positive pressure in the spray
 chamber exhaust tubing and drain bottle can affect 
 instrument performance and can _ contribute to excessive background
 
 contaminant levels. 
 8.13. The spray chamber exhaust and foreline pump exhaust must be vented with separate
 lengths of exhaust hose. These hoses can be connected into a common exhaust manifold.
 
 The separation of the exhaust minimizes the chances of foreline pump fluid
 vapor entering the spray chamber when drying gas is not flowing. 
 8.14 Ifanegative pressure vent is not available, the length of the tubing from the foreline pump
 
 and the drain bottle to the vent should each not _ exceed 
 460 cm (15 ft). 
 
 

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 8.15 Exhaust gas venting must comply with all local environmental codes. Health hazards
 include chemical toxicity of solvents, samples, buffers, pump fluid vapor, and aerosolized
 
 biological samples. 
 8.16 Operating environment 
 
 8.16.1 Mass Spectrometer Electrical Supply: 200 to 240 Vac, 50/60 Hz
 
 8.16.2 Mains supply voltage: Fluctuations not to exceed 10% of nominal supply
 voltage. Excessive fluctuations in the voltage of the power supply can create a
 shock hazard and can damage the instrument. 
 
 8.16.3 1260 HPLC system = 100-120 VAC with 15A supply circuit rating
 
 8.16.4 Do not use extension cords with the LC-MS instrument. Extension cords cannot
 supply enough power and can present a safety hazard. 
 8.16.5 Operating Temperature: 15°C to 35°C (59°F to 95°F) 
 
 8.16.6 Humidity: < 85% RH at 35°C, non-condensing, non-corrosive atmosphere
 
 9.0 Startup and Shutdown 
 
 9.1 System Startup 
 9.1.1 Perform this procedure to bring the system from the powered off state to standby
 
 mode. 
 9.1.2 The instrument should be properly installed with all power cables and gas lines
 connected. 
 
 9.1.3 Turn on power to the computer and monitor. 
 
 9.1.4 Check that the nitrogen gas supply is on and the supply pressure is 80 — 100 psi.
 
 9.159 Turn on the front power switch of the LC-MS instrument. The vacuum system
 automatically starts to pump down the instrument and the electronics are turned
 on. 
 
 9.2. System On/ System Standby 
 9.2.1 Perform this procedure when you need to switch between On and Standby
 modes. In Standby mode, source temperatures and gas flows are lowered but
 
 remain on to avoid contamination of the instrument. Standby mode is
 appropriate if the instrument will not be in use for up to one week.
 
 O22 
 Click the Data Acquisition icon on the desktop OR click Start > Agilent > Data
 Acquisition. 
 D223 In the Instrument Status pane, hover the cursor over the QQQ module. An On
 switch and an Off switch will appear. 
 
 

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 9.2.4 Select the appropriate switch to turn the system On or put it into Standby (Off).
 
 9.3. System Shutdown 
 9.3.1 Perform this procedure when you need to turn the instrument off for an extended
 
 period of time or when maintenance will be performed that requires a vacuum
 shutdown. 
 
 9.3.2 Click the Data Acquisition icon on the desktop OR click Start > Agilent > Data
 Acquisition. 
 
 9.3.3 In the Instrument Status pane, right-click on the QQQ module and select Vent.
 9.3.4 When the instrument has vented completely (High Vac reads 760 torr in the
 Actuals pane), toggle the power switch on the front of the instrument to turn it
 
 off. 
 10.0 Procedure for General Use 
 
 10.1 Click the Data Acquisition icon on the desktop OR click Start > Agilent > Data
 Acquisition. 
 
 10.2 The main window consists of multiple panes. You can show or hide a pane by using the
 commands in the View menu. You can drag a pane border to resize the pane. If you
 double-click the title bar of a pane, the pane “floats” outside of the main window. You
 
 can double-click the title bar again to “dock” the pane. 
 
 10.2.1 Instrument Status Pane 
 10.2.1.1 Shows the status of each device configured with the instrument
 (Error, Not Ready, Pre-run or Post-run, Running or Injecting, Idle,
 
 Offline, and Standby). 
 10.2.1.2 From the Status Pane, you can also set non-method control and
 configuration parameters for the LC devices and the MS instrument
 
 by using the right-click menu. 
 10.2.2 Actuals Pane 
 
 10.2.2.1. This pane shows the current value of selected instrument parameters.
 The parameters to be displayed can be configured using the right-
 
 click menu. 
 10.2.3 Chromatogram Plot Pane 
 
 10.2.3.1 This pane shows the chromatogram plot in real time.
 10.2.3.2 Instrument parameters can also be plotted in this pane.
 
 

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 10.2.3.3. The plots that are displayed can be configured in the QQQ tab in the
 Method Editor window. 
 
 10.2.4 Spectrum Pane 
 
 10.2.4.1 This pane shows the spectral plot in real time when you are acquiring
 data or tuning the instrument. 
 
 10.2.4.2 A separate tab is added for each detector configured on the
 instrument. 
 
 10.2.5 Method Editor Pane 
 10.2.5.1 In this pane, the acquisition parameters for the method can be set up.
 
 10.2.5.2 Checktune or Autotune can be run from the Autotune section of this
 pane. 
 
 10.2.6 Sample Run Pane 
 10.2.6.1 This pane allows the analysis of a single sample. 
 
 10.2.7. Worklist Pane 
 
 10.2.7.1 This pane allows the analysis of multiple samples. 
 
 10.3 Prepare the LC modules: 
 10.3.1 Switch the LC stream to Waste. 
 
 10.3.1.1 Inthe Instrument Status pane, right click the QQQ device.
 
 10.3.1.2 Select LC > Waste 
 10.3.2 Purge the LC pump and begin equilibrating the LC system to initial conditions
 of the method as outlined in D-807. 
 
 10.4 In the Actuals pane, set up to view real-time parameter values: 
 
 10.4.1 Right-click the Actuals pane, and select the Setup command.
 
 10.4.2 Add all parameters that you would like to monitor. 
 If desired, limits can be set for each parameter. If the parameter is outside of the
10.4.3 set limits, the background of the parameter will turn red.

 10.5 In the Chromatogram Plot pane, setup the signals to be monitored in real-time.
 
 10.5.1 Right-click the chromatogram plot, and click Change. 
 10.5.2 In the Edit Signal Plot dialog box, select the desired display signal.
 
 10.6 Perform Checktune or Autotune 
 
 10.6.1 Checktune should be performed at least once per week. 
 
 

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 10.6.2 Autotune should be performed at least once per month. 
 
 10.6.3 Click the QQQ tab in the Method Editor window. 
 
 10.6.4 Click the Autotune section in the left pane of the QQQ tab.
 Click the @ icon in the Autotune toolbar which locks the instrument for tuning.
10.6.5 Click the icon to perform checktune. Checktune takes approximately 3

10.6.6 minutes to run for each polarity.

 Click the “Y” icon to perform autotune. Autotune takes approximately 30
10.6.7 minutes.

 10.6.8 After checktune or autotune is complete, a tune report will be generated.
 
 10.6.9 If both Checktune and Autotune fail, check the progress box in the Tune status
 list to see why the tune failed. Then, either correct the problem or contact
 Agilent for technical support or service. 
 
 Click the Ff icon to unlock the instrument from Tune control.
10.6.10 10.7. Set up the Acquisition Method

 10.7.1 At the top of the Method Editor pane, select DA. 
 10.7.1.1 Click the Qual tab. 
 
 10.7.1.1.1. Ensure that the Qual Automation checkbox is not
 selected. 
 
 10.7.1.2 Click the Quant tab. 
 10.7.1.2.1 Ensure that the Quant Automation checkbox is not
 
 selected. 
 
 10.7.2 At the top of the Method Editor pane, select the Pump tab. 
 10.7.2.1. Enter the flow rate. 
 
 10.7.2.2 Enter the initial mobile phase conditions. 
 
 10.7.2.3 Enter the pressure limits. 
 10.7.2.4 Enter the Stoptime. 
 
 10.7.2.5 Select Posttime > Off 
 10.7.2.6 Enter parameters for each step of the mobile phase gradient in the
 
 Timetable. 
 10.7.3 At the top of the Method Editor pane, Select QQQ. 
 
 10.7.3.1 On the left, select Method > Acquisition. 
 
 

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 10.7.3.1.1 For each required time segment, select the Scan Type.
 
 10.7.3.1.2 For each required time segment, enter all Acquisition
 Parameters specified in the analyte specific method.
 
 10.7.3.2 On the left, select Method > Chromatograms. 
 10.7.3.2.1 Enter information for each chromatogram plot that
 
 should be displayed in the Chromatogram Plot pane.
 10.7.3.3 On the left, select Method > Timetable. 
 
 10.7.3.3.1 It is often useful to divert flow from the LC to waste
 when no peaks are eluting. This is done by entering the
 desired time in the timetable, and selecting Type >
 
 Diverter and then Value > To MS or To Waste.
 10.7.3.3.2 To switch flow from the LC to waste at the end of the
 run: select the “Post-run diverter position” check box,
 
 and “To waste”’. 
 
 10.7.4 Save the method. 
 10.7.4.1. All files related to a run (acquisition method, quantitation method,
 individual data files, report templates, etc.) should be stored under
 the D:\MassHunter\Data directory in analyte specific folders and
 
 organized by date. 
 10.7.4.2 Click Method > Save As or Method > Save. 
 
 10.8 Set up and run the samples. 
 
 10.8.1 In the Sample Run pane, click the Worklist tab at the bottom.
 
 10.8.2 Right-click the upper left corner of the worklist. 
 10.8.3 Click Add Multiple Samples. 
 
 10.8.4 Click the Sample Information tab, and enter the required information.
 Click the Sample Position tab, and specify the sample vial locations (ensure the
10.8.5 correct sample tray type has been configured by right-clicking the autosampler

 device image). 
 
10.8.6 Right-click the upper left corner of the worklist, and select Worklist Run

 Parameters. 
 On the Run Parameters tab, enter the correct path for the method.
10.8.7 10.8.8 Click the Data File Settings tab.

 10.8.9 Select the folders where the data files should be saved. 
 
 

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 10.8.10 Select the file naming options. 
 
 10.8.11 Click the Advanced Parameters tab, review the information, and click OK.
 10.8.12 To start the run click the G® or icons, or select Worklist > Run.
 
 10.9 After the run has completed, prepare the column for storage as outlined in D-807.
 
 10.10 Process the data. 
 10.10.1 Click the Quantitative Analysis © icon on the Desktop or start the program by
 
 selecting Programs > Agilent > MassHunter Workstation > Quantitative
 Analysis (QQQ) 
 
 10.10.2 Click File > New Batch. 
 10.10.3 Navigate to the folder that contains the data to be processed, and enter a name
 
 for the new batch. 
 10.10.4 Click Create Batch. 
 
 10.10.5 The Add Samples dialog box will appear. 
 
 10.10.6 Select the samples to be processed, and then click OK. 
 10.10.7 Ifa Quantitation Method already exists for the type of analysis being performed,
 
 open the method and adjust settings as necessary. 
 10.10.7.1 Click Method > Open. 
 
 10.10.7.2 Select Open Method from Existing Batch. 
 
 10.10.7.3 Select the batch containing the existing quantitation method, and
 then select Open. 
 10.10.7.4 In the Method Tasks pane, select Retention Time Setup. In the
 
 Method Table, adjust the retention time for each analyte-of-interest.
 10.10.7.5 In the Method Tasks pane, select Concentration Setup. Ensure that
 
 the standard concentrations listed in the Method Table are correct,
 or adjust as needed. 
 10.10.7.6 For existing methods, the integration parameters should generally
 
 not require adjustment. If necessary, adjust integration parameters
 from the Method Tasks pane under Advanced Tasks ~ Integration
 Parameters Setup. 
 
 10.10.7.7. After the quantitation method has been set up, select Exit from the
 Method Tasks pane. 
 
 10.10.7.8 Proceed to Section 10.10.9. 
 
 

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 LC-MS Operation Maintenance and Qualification D-802 1 
 
 10.10.8 Generate a Quantitation Method: 
 
 10.10.8.1 Click Method > Edit. 
 10.10.8.2 At the top of the Quantitative Analysis window, click New, and
 
 select New Method from Acquired MRM Data. 
 10.10.8.3 In the Dialog box, select a data file corresponding to a standard with
 
 high concentration of all target analytes, and click Open.
 10.10.8.4 Evaluate the automatically generated Quantitation Method for
 completeness/accuracy, and edit as required. 
 
 10.10.8.4.1 Under Method Setup Tasks in the left sidebar, click
 MRM Compound Setup. 
 
 For each qualifier ion listed in the Method Table:
 select the row containing the qualifier ion, right
 click the row, and select delete. Select Yes to
 
 delete the qualifier ion. 
 For each quantifier ion listed in the Method
 
 Table: select the row containing the quantifier
 ion, right click the row, and select New Qualifier.
 
 Select the correct product ion for the qualifier
 mass transition. 
 
 Adjust the Rel.Resp. until the ratio displayed in
 the Compound Information pane is near 100%.
 Ensure that the Uncertainty listed for the
 
 Qualifier Ion is correct. A value of 20 is typical.
 10.10.8.4.2 Under Method Setup Tasks in the left sidebar, click
 
 Method Setup Tasks > Retention Time Setup. 
 For each analyte, click the corresponding row,
 
 and ensure that the analyte retention times and
 deltas are correct. 
 
 10.10.8.4.3 Under Method Setup Tasks in the left sidebar, click
 Method Setup Tasks > ISTD Setup. 
 For each target analyte, ensure that the ISTD is
 
 correct. If not correct, click the down arrow in the
 ISTD Compound Name cell and select the correct
 ISTD. 
 
 

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 For each ISTD, enter the ISTD concentration. If
 the concentration is the same for all samples, a
 value of 1 is sufficient. 
 
 10.10.8.4.4 Under Method Setup Tasks in the left sidebar, click
 Method Setup Tasks > Concentration Setup. 
 
 For the first target analyte, select the
 corresponding row, right click the row, and select
 
 New Calibration Level. 
 Enter the level name (typically L1, L2, etc.) and
 
 enter the level concentration in units appropriate
 to generate the final result in the correct units
 (generally mcg/mL). If the product formula
 contains the target analyte in a form that is
 different from the reference standard (e.g. the
 
 formula contains thiamine mononitrate while the
 reference standard is thiamine hydrochloride),
 the number entered should reflect the working
 standard concentration in terms of the form that
 is present in the product profile. Calculation of
 
 the working standard concentration should be
 documented in the laboratory notebook. 
 
 Repeat for each required calibration level.
 If other analytes share the same concentration
 
 levels, click Method > Copy Calibration Levels
 To ..., then select the analytes to copy the levels
 to, then click OK. 
 
 If other analytes have different concentration
 levels, repeat the process for each analyte.
 
 Select the correct units for each analyte in the
 Units column. 
 
 10.10.8.4.5 Under Method Setup Tasks in the left sidebar, click
 Method Setup Tasks > Calibration Curve Setup.
 Inspect and/or correct the CF, CF Origin, and CF
 
 Weight columns. 
 10.10.8.4.6 Under Advanced Tasks in the left sidebar, click
 
 Advanced Tasks > Integration Parameters Setup.
 
 

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 ® In the method table, select the row for each
 analyte and ensure that the peak is properly
 
 integrated by viewing the chromatogram in the
 Compound Information pane. If necessary,
 correct the integration by adjusting the Int. and
 Int. Params. settings. 
 
 10.10.8.5 Click Validate to validate the method setup, and correct any errors
 or warnings that are found. 
 
 10.10.8.6 Ifno errors or warnings are found, click Exit. 
 
 10.10.8.7 Click Yes to apply the method to the batch. 
 10.10.9 Enter the sample amount for each sample in the Amt. column of the batch table.
 Units should be appropriately selected to generate the final result in the correct
 
 units. 
 10.10.10 Enter the sample dilution for each sample in the Dil. column of the batch table.
 
 Units should be appropriately selected to generate the final result in the correct
 units. If multiple dilutions were performed, this value should include all
 dilutions. For example, if the sample was dissolved in 50 mL and then diluted
 1/10, the dilution would be 0.5 L. 
 
 10.10.11 Enter the weight of a single dosage unit from the product profile for each sample
 in the Tot. Amt. column of the Batch Table. Units should be appropriately
 selected to generate the final result in the correct units. 
 
 10.10.12 Click the = Aus") icon to start data processing. 
 
 10.10.13 After processing is complete, click File > Save Batch. 
 
 10.11 Review the integration 
 10.11.1 Click the first row of the Batch Table. 
 
 10.11.2 Review the integration for the current analyte by viewing the chromatogram in
 the Compound Information pane. 
 
 10.11.3 Use the Next Sample icon V at the top of the batch table to review integration
 for the current analyte in all samples. 
 
 10.11.4 Use the Next Compound icon > at the top of the batch table to review integration
 for all analytes. 
 10.11.5 If any chromatograms are not properly integrated, return to Integration
 
 Parameters Setup (Section 10.10.8.4.6) to make adjustments. 
 10.12 Review the Calibration 
 
 

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 10.12.1 After processing, the batch table will be highlighted with flags and/or colors to
 indicate lines that contain any problem. Hover the cursor over the highlighted
 cell to show an explanation of the problem. 
 
 10.12.2 Make sure the Batch Table is set to single compound display mode by clicking
 the Single Compound/Sample View icon above the batch table. 
 
 10,12:3 For each calibration injection, change the sample type to Cal.
 
 10.12.4 For each calibration injection, select the correct level name by clicking the drop
 down box in the Level column. 
 
 10.12.5 Click Home > Analyze Batch. 
 10.12.6 Review the calibration curve for each analyte. 
 
 10.12.7 Ensure that the coefficient of determination (R*) for the calibration of each
 analyte meets the acceptance criteria listed in the test method.
 
 10.12.8 Click Next Compound in the batch toolbar to cycle through each analyte.
 
 10.13 Generate a report 
 10.13.1 Near the top of the screen on the Home tab, select Edit Report Method.
 
 10.13.2 Click Add Template, and select the desired report template.
 
 10.13.3 Click Save and Exit, then enter a filename to save the method as.
 10.13.4 Click Generate Report. 
 
 10.13.5 Select the QuantReports folder. 
 
 10.13.6 Select the Report Method that was previously saved. 
 10.13.7 Press OK. 
 
 11.0 Preventative Maintenance 
 
 11.1 Refer to D-807 HPLC Operation, Maintenance, and Qualification for preventative
 maintenance of the HPLC portion of the LC-MS system. 
 
 11.2 Refer to the electronic help, which can be accessed from the Windows Start Menu by
 selecting Agilent > Ultivo LC-TQ Resources and then choosing Mass Spectrometer >
 Maintenance Guide, for instructions on how to perform regular maintenance on the LC-
 
 MS system. 
 12.0 Consumables 
 
 12.1. ESI-L Calibrant Solution, Agilent Part # G1969-85000 
 
 12.2 Abrasive mesh, Agilent Part # 8660-0827 
 
 

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 12.3. Cotton swabs, Agilent Part # 5080-5400 
 12.4 SW60 foreline pump oil, Agilent Part # 6040-1361 
 
 12.5 Capillary 90, Agilent Part # G6303-80004 
 
 12.6 Canted Coil Spring, Agilent Part # G1460-2571 
 12.7. %-inch ID front capillary seal, Agilent Part # 0905-1475 
 
 12.8 Agilent Jet Stream heater replacement kit, Agilent Part # G1958-68000
 
 12.9 Nebulizer (needle SS316 replacement) kit for Agilent Jet Stream, Agilent Part # G1958-
 60137. 
 
 13.0 Performance Qualification 
 
 13.1 The following tests are recommended for annual performance qualification (PQ) of the
 Ultivo mass spectrometer. For guidance on PQ of the HPLC system connected to the
 mass spectrometer, refer to D-807 HPLC Operation, Maintenance, and Qualification.
 
 13.2 Supplies needed 
 13.2.1 OQPV Sulfa Standard for LCMS (Agilent Part No. 5190-0580) 
 
 13.2.2 ESI-L Low Concentration Tuning Mix (Agilent Part No. G1969-85000)
 
 13.2.3 Methanol (LC-MS grade) 
 13.2.4 Water (©18MQ:ecm) 
 
 13.2.5 C18 HPLC column (select dimensions to result in acceptable peak shape and
 separation of all components in the Sulfa Standard) 
 
 13.3 Vacuum Verification 
 
 13.3.1 A stable, high vacuum is required for high-sensitivity mass spectrometry.
 13.3.2 Passing the vacuum verification is a pre-requisite for all other PQ tests listed in
 
 this procedure. 
 13.3.3 With the instrument in the Standby state, take five readings of the QQQ High
 Vac parameter over the course of 10 minutes. The parameter is located in the
 
 MassHunter Data Acquisition application in the Actuals pane.
 13.3.4 Acceptance Criteria: 
 
 13.3.4.1 The mean High Vac reading is NMT 5.0x10° torr. 
 
 13.4 Mass Accuracy Verification 
 13.4.1. The built-in autotune function is performed to ensure proper mass accuracy of
 the mass spectrometer. 
 
 

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 13.4.2. Perform autotune of the instrument: 
 
 13.4.2.1 Ensure that there is sufficient ESI-L Low Concentration Tuning Mix
 in the bottle located at the front right side of the mass spectrometer.
 13.4.2.2 In the method editor pane, click on the QQQ tab. 
 
 13.4.2.3 Select Tune > Autotune. 
 
 Click the ff icon in the Autotune toolbar which locks the instrument
13.4.2.4 for tuning.

 Click the ‘Y” icon to perform autotune. Autotune takes
13.4.2.5 approximately 30 minutes.

 13.4.2.6 After autotune is complete, a tune report will be generated.
 
 Click the on icon to unlock the instrument from Tune control.
13.4.2.7 13.4.3. Acceptance Criteria:

 13.4.3.1 Positive Mode: 
 
 13.4.3.1.1 Mass 1 = 117.89 — 118.29 
 
 13.4.3.1.2 Mass 2 = 321.85 — 322.25 
 13.4.3.1.3. Mass 3 = 621.83 — 622.23 
 
 13.4.3.1.4 Mass 4= 921.81 — 922.21 
 
 13.4.3.1.5 Mas5s = 1221.79— 1222.19 
 13.4.3.2 Negative Mode: 
 
 13.4.3.2.1 Mass 1 = 112.79— 113.19 
 
 13.4.3.2.2 Mass 2 = 301.80 — 302.20 
 13.4.3.2.3 Mass 3 = 601.78 — 602.18 
 
 13.4.3.2.4 Mass 4 = 1033.79 — 1034.19 
 
 13.4.3.2.5 Mass 5 = 1333.77 — 1334.17 
 13.5 Instrument Method Parameters 
 
 13.5.1 For the remaining tests, set up an acquisition method with the following
 parameters: 
 
 13.5.2 Sampler 
 
 13.5.2.1 Injection Volume: 1 nL 
 [3.5.2.2 Enable Needle Wash: Selected 
 
 

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 Standard Operating Procedure SOP No Rev 
 Page 16 of 18 
 LC-MS Operation Maintenance and Qualification D-802 
 
 13.5.2.3. Mode: Flush Port 
 13.5.2.4 Time: 10 sec 
 
 13.5.3. Binary Pump 
 
 13.5.3.1 Flow Rate: adjust to result in pressure of 100 bar — 250 bar and
 retention time less than 1 minute depending on the column used.
 
 13.5.3.2. Mobile Phase: H2O/methanol (25/75) 
 13.5.3.3 Stoptime: 1.0 min 
 
 13.5.4 Column Oven 
 
 13.5.4.1 Temperature: 40 °C 
 13.5.5 QQQ 
 
 13.5.5.1 Acquisition 
 
 13.5.5.1.1 Ion Source: AJS ESI 
 13.5.5.1.2 Scan type: MRM 
 
 13.5.5.1.3 Polarity: Positive 
 
 13.5.5.1.4 Acquisition Parameters 
 RT “ : Precurso MS2 |Product| Dwell | Frag 
 Analyte ISTD (min) Window Mbt Res r(m/z)| Res | (m/z) | (ms) (Vv) CE (V)
 
 (min) 
 
 sulfadimethoxine no 0.5 1.0 Unit | 311.0 | Unit 156.0 200 150 24 
 
 13.5.5.2 Source Parameters 
 
 13.5.5.2.1 Ion Source: AJS ESI 
 
 13.5.3.2.2 Gas Temperature: 250 °C 
 13.5.5.2.3 Gas Flow: 12.0 L/min 
 
 13.5.5.2.4 Nebulizer Pressure: 35 psi 
 
 13.5.5.2.5 Sheath Gas Temperature: 400 °C 
 13..5.5.2.6 Sheath Gas Flow: 11.0 L/min 
 
 13.5.5.2.7 Capillary Voltage (Positive Setpoint): 3000 V
 
 13.5.5.2.8 Nozzle Voltage (Positive Setpoint): 0 V 
 13.6 Linearity 
 
 

[SOP 

 Standard Operating Procedure SOP No | Rev 
 LC-MS Operation Maintenance and Qualification D-802 fof BEER EME ES 
 
 13.6.1 The linearity test uses the Sulfa Standard to evaluate response linearity.
 13.6.2 Connect a suitable column, and equilibrate the LC system with H2O/methanol
 (25/75) and at a flow rate that results in pressure in the range 100 bar — 250 bar.
 
 13.6.3 Perform at least three blank injections followed by a single 1 L injection at each
 of five concentrations: 0.0100, 0.0250, 0.100, 0.500, and 1.00 mcg/mL.
 
 13.6.4 Plot peak area of the sulfadimethoxine peak (m/z 156) versus concentration.
 
 13.6.5 Perform linear regression of the data using the method of least-squares.
 
 13.6.6 Acceptance Criteria: 
 13.6.6.1 The coefficient of determination (R*) is NLT 0.980.
 
 13.7. Precision 
 
 13.7.1 The precision test uses the Sulfa Standard to evaluate instrument precision.
 13.7.2 Connect a suitable column, and equilibrate the LC system with H2O/methanol
 (25/75) and at a flow rate that results in pressure in the range 100 bar — 250 bar.
 
 13.7.3 Perform at least three blank injections followed by six replicate 1 uL injections
 of the 0.0100 mcg/mL Sulfa Standard. 
 
 13.7.4 Measure the peak area of the sulfadimethoxine (m/z 156) peak in the replicate
 injections. 
 
 13.7.5 Acceptance Criteria: 
 
 13.7.5.1 The %RSD of the sulfadimethoxine peak area in the six replicate
 injections is NMT 10.0%. 
 
 13.8 Carry-Over 
 13.8.1 The carry-over test uses the Sulfa Standard to evaluate instrument carry-over.
 
 13.8.2 Connect a suitable column, and equilibrate the LC system with H2O/methanol
 (25/75) and at a flow rate that results in pressure in the range 100 bar — 250 bar.
 
 13.8.3 Perform at least three blank injections followed by a single 1 wL injection of the
 1.00 mcg/mL Sulfa Standard and then a blank injection. 
 
 13.8.4 Calculate the amount of carry-over by dividing the peak area of the
 sulfadimethoxine peak (m/z 156) measured in the blank injection by the peak
 area of the sulfadimethoxine peak measured in the 1.00 mcg/mL Sulfa Standard.
 Multiply the carry-over result by 100 to obtain the value in percent format.
 
 13.8.5 Acceptance Criteria: 
 
 13.8.5.1 Carry-over is NMT 1.00%. 
 
 

[SOP 

 LC-MS Ope S r t a a t n i d ° o ar n d M O a p i e n° r t a e t n in a g n c P e ro a c n ed d u Q r u e a lif. icati. on S D O - P 80 N 2 o | Re 1 v Page. ES.0F 15
 
 13.9 Signal-to-Noise 
 13.9.1 The signal-to-noise test uses the Sulfa Standard to evaluate signal-to-noise.
 
 13.9.2 Connect a suitable column, and equilibrate the LC system with H2O/methanol
 (25/75) and at a flow rate that results in pressure in the range 100 bar — 250 bar.
 
 13.9.3 Perform at least three blank injections followed by a single 1 wL injection of the
 0.01 mcg/mL Sulfa Standard. 
 
 13.9.4 Calculate the signal-to-noise ratio for the sulfadimethoxine peak (m/z 156)
 using MassHunter software. 
 
 13.9.5 Acceptance Criteria: 
 13.10 Signal-to-Noise is NLT 1000. 
 
 14.0 Revision History 

| Rev | Date | Description of Changes | CCR # | By |
|-----|----------|------------------------|-------|----|
| 0 | 04/05/21 | New Document N/A S. Sassman | - | - |

 Add performance qualification section, remove things that don’t
 i 10/28/21 CC-21-0401 | S. Sassman 
 apply to system, edit for clarification of meaning.